Hydrolysis & Biodegradability

01Hydrolysis & Biodegradability

Polyester hydrolysis

This section covers how acid or alkali hydrolysis breaks ester links in polyesters to form smaller molecules.

Breaking ester links

Polyesters contain ester links, COO\ce{-COO-}, within their main chains. These links can be broken by hydrolysis, dividing a long polymer molecule into smaller fragments.

Hydrolysis restores alcohol-derived and carboxyl-derived groups at the point where an ester link is broken. The exact form of the carboxyl-containing product depends on whether the conditions are acidic or alkaline.

The hydrolysable functional group is the ester linkage:

COO\ce{-COO-}

Repeated cleavage of these links can eventually produce compounds corresponding to the monomers used to make the polyester.

RCOOR0H+(aq)RCOOH+HOR0

Acid and alkaline hydrolysis

Polyesters can be hydrolysed using aqueous acid or aqueous alkali. The two conditions give different forms of the acid-derived product.

Conditions Products from an ester link
Aqueous acid Carboxylic acid group + alcohol group
Aqueous alkali Carboxylate salt group + alcohol group

Complete hydrolysis of a polyester made from a dicarboxylic acid and a diol therefore gives fragments corresponding to those original monomers, although the acid-derived groups are present as carboxylate salts under alkaline conditions.

Exam Tip: Check the conditions before drawing the products. Under acidic conditions, restore a carboxylic acid and an alcohol; under alkaline conditions, show a carboxylate salt and an alcohol.

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